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D. A. Fink et al.; 15 págs.; 17 figs.; 3 tabs.; Open Access funded by Creative Commons Atribution Licence 3.0 ; A Laser Ion Source and Trap (LIST) for a thick-target, isotope-separation on-line facility has been implemented at CERN ISOLDE for the production of pure, laser-ionized, radioactive ion beams. It offers two modes of operation, either as an ion guide, which performs similarly to the standard ISOLDE resonance ionization laser ion source (RILIS), or as a more selective ion source, where surface-ionized ions from the hot ion-source cavity are repelled by an electrode, while laser ionization is done within a radiofrequency quadrupole ion guide. The first physics application of the LIST enables the suppression of francium contamination in ion beams of neutron-rich polonium isotopes at ISOLDE by more than 1000 with a reduction in laser-ionization efficiency of only 20. Resonance ionization spectroscopy is performed directly inside the LIST device, allowing the study of the hyperfine structure and isotope shift of 217Po for the first time. Nuclear decay spectroscopy of 219Po is performed for the first time, revealing its half-life, α- to-β-decay branching ratio, and α-particle energy. This experiment demonstrates the applicability of the LIST at radioactive ion-beam facilities for the production and study of pure beams of exotic isotopes. Published by the American Physical Society ; This work was supported by the Bundesministerium für Bildung und Forschung (BMBF, Germany) within the Wolfgang- Gentner programme as well as through the consecutive project fundings of 06Mz9181I, 06Mz7177D, and 05P12UMCIA, by FWO-Vlaanderen (Belgium), by GOA/2010/010 (BOF-KULeuven), by the IUAP-Belgian State Belgian Science Policy (BRIX network P7/12), by the U.K. Science and Technology Facilities Council (STFC), by the European Union within FP7 (ENSAR No. 262010), by the Slovak Research and Development Agency (Contract No. APVV-0105-10), by the Slovak grant agency VEGA, and the Reimei Foundation of JAEA (Contract No. 1/0576/13). T. E. C. was supported by STFC Ernest Rutherford Grant No. ST/J004189/1. ; Peer Reviewed

13 pags., 7 figs., 3 tabs. ; A new β-decaying state in Bi214 has been identified at the ISOLDE Decay Station at the CERN-ISOLDE facility. A preferred Iπ=(8-) assignment was suggested for this state based on the β-decay feeding pattern to levels in Po214 and shell-model calculations. The half-life of the Iπ=(8-) state was deduced to be T1/2=9.39(10) min. The deexcitation of the levels populated in Po214 by the β decay of this state was investigated via γ-γ coincidences and a number of new levels and transitions was identified. Shell-model calculations for excited states in Bi214 and Po214 were performed using two different effective interactions: the H208 and the modified Kuo-Herling particle interaction. Both calculations agree on the interpretation of the new β-decaying state as an Iπ=8- isomer and allow for tentative assignment of shell-model states to several high-spin states in Po214. ; This work has been supported by the Research Foundation Flanders (FWO, Belgium), by GOA/2015/010 (BOF KU Leuven), the Interuniversity Attraction Poles Programme initiated by the Belgian Science Policy Office (BriX network P7/12), by the ENSAR2: European Union's Horizon 2020 research and innovation programme under Grant Agreement No. 654002, by the U.K. Science and Technology Facilities Council, by the Slovak Research and Development Agency (Contract No. APVV-18-0268), by the Slovak grant agency VEGA (Contract No. 1/0651/21), by RFBR according to the research project N 19-02-00005, by the Romanian IFA Grant CERN/ISOLDE, by the Spanish Funding Agency (AEI) under the project PID2019-104390GB-I00, by the German BMBF under Grant No. 05P18PKCIA and by the Spanish Ministerio de Ciencia e Innovación grant PID2019-104714GB-C21. M.S. acknowledges funding from the European Union's Horizon 2020 research and innovation program under Grant Agreement No. 771036 (ERC CoG MAIDEN). ; Peer reviewed