Mechanism of magnetic transition in FeCrCoNi-based high entropy alloys
In: Materials and design, Band 103, S. 71-74
ISSN: 1873-4197
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In: Materials and design, Band 103, S. 71-74
ISSN: 1873-4197
The skyrmion racetrack is a promising concept for future information technology. There, binary bits are carried by nanoscale spin swirls–skyrmions–driven along magnetic strips. Stability of the skyrmions is a critical issue for realising this technology. Here we demonstrate that the racetrack skyrmion lifetime can be calculated from first principles as a function of temperature, magnetic field and track width. Our method combines harmonic transition state theory extended to include Goldstone modes, with an atomistic spin Hamiltonian parametrized from density functional theory calculations. We demonstrate that two annihilation mechanisms contribute to the skyrmion stability: At low external magnetic field, escape through the track boundary prevails, but a crossover field exists, above which the collapse in the interior becomes dominant. Considering a Pd/Fe bilayer on an Ir(111) substrate as a well-established model system, the calculated skyrmion lifetime is found to be consistent with reported experimental measurements. Our simulations also show that the Arrhenius pre-exponential factor of escape depends only weakly on the external magnetic field, whereas the pre-exponential factor for collapse is strongly field dependent. Our results open the door for predictive simulations, free from empirical parameters, to aid the design of skyrmion-based information technology. ; e acknowledge financial support from the Icelandic Research Fund (Grant No. 163048-052), the mega-grant of the Ministry of Education and Science of the Russian Federation (grant no. 14. Y26.31.0015), Göran Gustafsson Foundation, the Russian Foundation for Basic Research (Grant No. 18-02-00267 A), Vetenskapsrådet (VR), Carl Tryggers Stiftelse (CTS), the European Union's Horizon 2020 research and innovation programme (grant agreement no. 665095–FET-Open project MAGicSky), Academy of Finland (grant no. 278260), and SwedishEnergy Agency (STEM). Calculations of skyrmion lifetimes were supported by the Russian Science Foundation (Grant No. 17-72-10195). Some of the computations were performed on resources provided by the Swedish National Infrastructure for Computing (SNIC) at the National Supercomputer Center (NSC), Linköping University, the PDC Centre for High Performance Computing (PDC-HPC), KTH, and the High Performance Computing Center North (HPC2N), Umeå University. ; Peer Reviewed
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