Suchergebnisse

D. A. Fink et al.; 15 págs.; 17 figs.; 3 tabs.; Open Access funded by Creative Commons Atribution Licence 3.0 ; A Laser Ion Source and Trap (LIST) for a thick-target, isotope-separation on-line facility has been implemented at CERN ISOLDE for the production of pure, laser-ionized, radioactive ion beams. It offers two modes of operation, either as an ion guide, which performs similarly to the standard ISOLDE resonance ionization laser ion source (RILIS), or as a more selective ion source, where surface-ionized ions from the hot ion-source cavity are repelled by an electrode, while laser ionization is done within a radiofrequency quadrupole ion guide. The first physics application of the LIST enables the suppression of francium contamination in ion beams of neutron-rich polonium isotopes at ISOLDE by more than 1000 with a reduction in laser-ionization efficiency of only 20. Resonance ionization spectroscopy is performed directly inside the LIST device, allowing the study of the hyperfine structure and isotope shift of 217Po for the first time. Nuclear decay spectroscopy of 219Po is performed for the first time, revealing its half-life, α- to-β-decay branching ratio, and α-particle energy. This experiment demonstrates the applicability of the LIST at radioactive ion-beam facilities for the production and study of pure beams of exotic isotopes. Published by the American Physical Society ; This work was supported by the Bundesministerium für Bildung und Forschung (BMBF, Germany) within the Wolfgang- Gentner programme as well as through the consecutive project fundings of 06Mz9181I, 06Mz7177D, and 05P12UMCIA, by FWO-Vlaanderen (Belgium), by GOA/2010/010 (BOF-KULeuven), by the IUAP-Belgian State Belgian Science Policy (BRIX network P7/12), by the U.K. Science and Technology Facilities Council (STFC), by the European Union within FP7 (ENSAR No. 262010), by the Slovak Research and Development Agency (Contract No. APVV-0105-10), by the Slovak grant agency VEGA, and the Reimei Foundation of JAEA (Contract No. 1/0576/13). T. E. C. was supported by STFC Ernest Rutherford Grant No. ST/J004189/1. ; Peer Reviewed

The β−-particle-emitting erbium-169 is a potential radionuclide toward therapy of metastasized cancer diseases. It can be produced in nuclear research reactors, irradiating isotopically-enriched 168Er2O3. This path, however, is not suitable for receptor-targeted radionuclide therapy, where high specific molar activities are required. In this study, an electromagnetic isotope separation technique was applied after neutron irradiation to boost the specific activity by separating 169Er from 168Er targets. The separation efficiency increased up to 0.5% using resonant laser ionization. A subsequent chemical purification process was developed as well as activity standardization of the radionuclidically pure 169Er. The quality of the 169Er product permitted radiolabeling and pre-clinical studies. A preliminary in vitro experiment was accomplished, using a 169Er-PSMA-617, to show the potential of 169Er to reduce tumor cell viability. © Copyright © 2021 Talip, Borgna, Müller, Ulrich, Duchemin, Ramos, Stora, Köster, Nedjadi, Gadelshin, Fedosseev, Juget, Bailat, Fankhauser, Wilkins, Lambert, Marsh, Fedorov, Chevallay, Fernier, Schibli and van der Meulen. ; The authors thank CERN ISOLDE and RILIS teams for the laser operation (Maxim D. Seliverstov, Katerina Chrysalidis), radiation protection and logistic teams of PSI (Tobias Schneider) and CERN (Alexandre Dorsival, Matthieu Deschamps and Elodie Aubert, Philippe Bertreix, Nicolas Riggaz, Nabil Menaa, Aurore Boscher, Jeremie Comte, Benjamin Juif); the LARISSA workgroup of Mainz University for the laser preparation and erbium laser ionization scheme development (Prof. Dr. Klaus Wendt and Dr. Dominik Studer). The authors are grateful to Fan Sozzi-Guo, Muhamet Djelili, Alexander V?gele and Walter Hirzel (PSI) and Bernard Cr?pieux, Giacomo Lunghi, Francesco Riccardi, Miranda Van Stenis, Thomas Schneider (CERN) for technical support. Funding. ZT and NM received funding from the Swiss National Science Foundation (SNF Grant Number: 200021_188495). CM obtained funding for this project from the Swiss Cancer Research (KFS-4678-02-2019-R). FB received funding from the European Union's Horizon 2020 research and innovation programme under the Marie Sk?odowska-Curie Grant Agreement No 701647.

13 pags., 7 figs., 3 tabs. ; A new β-decaying state in Bi214 has been identified at the ISOLDE Decay Station at the CERN-ISOLDE facility. A preferred Iπ=(8-) assignment was suggested for this state based on the β-decay feeding pattern to levels in Po214 and shell-model calculations. The half-life of the Iπ=(8-) state was deduced to be T1/2=9.39(10) min. The deexcitation of the levels populated in Po214 by the β decay of this state was investigated via γ-γ coincidences and a number of new levels and transitions was identified. Shell-model calculations for excited states in Bi214 and Po214 were performed using two different effective interactions: the H208 and the modified Kuo-Herling particle interaction. Both calculations agree on the interpretation of the new β-decaying state as an Iπ=8- isomer and allow for tentative assignment of shell-model states to several high-spin states in Po214. ; This work has been supported by the Research Foundation Flanders (FWO, Belgium), by GOA/2015/010 (BOF KU Leuven), the Interuniversity Attraction Poles Programme initiated by the Belgian Science Policy Office (BriX network P7/12), by the ENSAR2: European Union's Horizon 2020 research and innovation programme under Grant Agreement No. 654002, by the U.K. Science and Technology Facilities Council, by the Slovak Research and Development Agency (Contract No. APVV-18-0268), by the Slovak grant agency VEGA (Contract No. 1/0651/21), by RFBR according to the research project N 19-02-00005, by the Romanian IFA Grant CERN/ISOLDE, by the Spanish Funding Agency (AEI) under the project PID2019-104390GB-I00, by the German BMBF under Grant No. 05P18PKCIA and by the Spanish Ministerio de Ciencia e Innovación grant PID2019-104714GB-C21. M.S. acknowledges funding from the European Union's Horizon 2020 research and innovation program under Grant Agreement No. 771036 (ERC CoG MAIDEN). ; Peer reviewed

10 pags., 8 figs., 1 tab.-- Open Access funded by Creative Commons Atribution Licence 4.0 ; Excited states in Sn133 were investigated through the ß decay of In133 at the ISOLDE facility. The ISOLDE Resonance Ionization Laser Ion Source (RILIS) provided isomer-selective ionization for In133, allowing us to study separately, and in detail, the ß-decay branch of In133J¿=(9/2+) ground state and its J¿=(1/2-) isomer. Thanks to the large spin difference of the two ß-decaying states of In133, it is possible to investigate separately the lower and higher spin states in the daughter, Sn133, and thus to probe independently different single-particle and single-hole levels. We report here new ¿ transitions observed in the decay of In133, including those assigned to the deexcitation of the neutron-unbound states. ; We acknowledge the support of the ISOLDE Collaboration and technical teams. This work was supported in part by the Polish National Science Center under Contract No. UMO-2015/18/E/ST2/00217 and under Contract No. UMO-2015/18/M/ST2/00523, by the Spanish MINECO via FPA2015-65035-P project, by the Portuguese FCT via CERN/FIS-NUC/0004/2015 and CERN-FIS-PAR-0005-2017 projects. The research leading to these results has received funding from the European Union's Horizon 2020 research and innovation programme under Grant Agreement No. 654002.