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D. A. Fink et al.; 15 págs.; 17 figs.; 3 tabs.; Open Access funded by Creative Commons Atribution Licence 3.0 ; A Laser Ion Source and Trap (LIST) for a thick-target, isotope-separation on-line facility has been implemented at CERN ISOLDE for the production of pure, laser-ionized, radioactive ion beams. It offers two modes of operation, either as an ion guide, which performs similarly to the standard ISOLDE resonance ionization laser ion source (RILIS), or as a more selective ion source, where surface-ionized ions from the hot ion-source cavity are repelled by an electrode, while laser ionization is done within a radiofrequency quadrupole ion guide. The first physics application of the LIST enables the suppression of francium contamination in ion beams of neutron-rich polonium isotopes at ISOLDE by more than 1000 with a reduction in laser-ionization efficiency of only 20. Resonance ionization spectroscopy is performed directly inside the LIST device, allowing the study of the hyperfine structure and isotope shift of 217Po for the first time. Nuclear decay spectroscopy of 219Po is performed for the first time, revealing its half-life, α- to-β-decay branching ratio, and α-particle energy. This experiment demonstrates the applicability of the LIST at radioactive ion-beam facilities for the production and study of pure beams of exotic isotopes. Published by the American Physical Society ; This work was supported by the Bundesministerium für Bildung und Forschung (BMBF, Germany) within the Wolfgang- Gentner programme as well as through the consecutive project fundings of 06Mz9181I, 06Mz7177D, and 05P12UMCIA, by FWO-Vlaanderen (Belgium), by GOA/2010/010 (BOF-KULeuven), by the IUAP-Belgian State Belgian Science Policy (BRIX network P7/12), by the U.K. Science and Technology Facilities Council (STFC), by the European Union within FP7 (ENSAR No. 262010), by the Slovak Research and Development Agency (Contract No. APVV-0105-10), by the Slovak grant agency VEGA, and the Reimei Foundation of JAEA (Contract No. 1/0576/13). T. E. C. was supported by STFC Ernest Rutherford Grant No. ST/J004189/1. ; Peer Reviewed