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13 pags., 5 figs., 2 tabs. ; The structure of Po208 populated through the EC/β+ decay of At208 is investigated using γ-ray spectroscopy at the ISOLDE Decay Station. The presented level scheme contains 27 new excited states and 43 new transitions, as well as a further 50 previously observed γ rays which have been (re)assigned a position. The level scheme is compared to shell model calculations. Through this analysis approximately half of the β-decay strength of At208 is found to proceed via allowed decay and half via first-forbidden decay. The first-forbidden transitions predominantly populate core excited states at high excitation energies, which is qualitatively understood using shell model considerations. This mass region provides an excellent testing ground for the competition between allowed and first-forbidden β-decay calculations, important for the detailed understanding of the nucleosynthesis of heavy elements. ; The research leading to these results received funding from the European Union's Horizon 2020 research and innovation program under Grant Agreement No. 654002. Support from the European Union Seventh Framework through ENSAR Contract No. 262010, as well as the Science and Technology Facilities Council (U.K.) through Grants No. ST/P005314/1, No. ST/L005743/1, No. ST/J000051/1, No. ST/L005670/1, and No. ST/P004598/1, the German BMBF under Contract No. 05P18PKCIA and "Verbundprojekt 05P2018" as well as Spanish MINECO Grants No. FPA2015-65035- P and No. FPA2017-87568-P, FWO Vlaanderen (Belgium), GOA/2015/010 (BOF KU Leuven), the Excellence of Science Programme (EOS-FWO), the Interuniversity Attraction Poles Programme initiated by the Belgian Science Policy Office (BriX network P7/12), the Polish National Science Centre under Contracts No. UMO-2015/18/M/ST2/00523 and No. UMO-2019/33/N/ST2/03023, National Science Foundation (U.S.) Grant No. PHY1811855, and the Romanian IFA project CERN-RO/ISOLDE is acknowledged. P.H.R. acknowledges support from the U.K. Department for Business, Energy and Industrial Strategy via the National Measurement Office ; Peer reviewed

13 pags., 7 figs., 3 tabs. ; A new β-decaying state in Bi214 has been identified at the ISOLDE Decay Station at the CERN-ISOLDE facility. A preferred Iπ=(8-) assignment was suggested for this state based on the β-decay feeding pattern to levels in Po214 and shell-model calculations. The half-life of the Iπ=(8-) state was deduced to be T1/2=9.39(10) min. The deexcitation of the levels populated in Po214 by the β decay of this state was investigated via γ-γ coincidences and a number of new levels and transitions was identified. Shell-model calculations for excited states in Bi214 and Po214 were performed using two different effective interactions: the H208 and the modified Kuo-Herling particle interaction. Both calculations agree on the interpretation of the new β-decaying state as an Iπ=8- isomer and allow for tentative assignment of shell-model states to several high-spin states in Po214. ; This work has been supported by the Research Foundation Flanders (FWO, Belgium), by GOA/2015/010 (BOF KU Leuven), the Interuniversity Attraction Poles Programme initiated by the Belgian Science Policy Office (BriX network P7/12), by the ENSAR2: European Union's Horizon 2020 research and innovation programme under Grant Agreement No. 654002, by the U.K. Science and Technology Facilities Council, by the Slovak Research and Development Agency (Contract No. APVV-18-0268), by the Slovak grant agency VEGA (Contract No. 1/0651/21), by RFBR according to the research project N 19-02-00005, by the Romanian IFA Grant CERN/ISOLDE, by the Spanish Funding Agency (AEI) under the project PID2019-104390GB-I00, by the German BMBF under Grant No. 05P18PKCIA and by the Spanish Ministerio de Ciencia e Innovación grant PID2019-104714GB-C21. M.S. acknowledges funding from the European Union's Horizon 2020 research and innovation program under Grant Agreement No. 771036 (ERC CoG MAIDEN). ; Peer reviewed