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4 páginas, 4 figuras.-- El Pdf es la versión pre-print.-- et al. ; Shell structure and magic numbers in atomic nuclei were generally explained by pioneering work that introduced a strong spin–orbit interaction to the nuclear shell model potential. However, knowledge of nuclear forces and the mechanisms governing the structure of nuclei, in particular far from stability, is still incomplete. In nuclei with equal neutron and proton numbers (N = Z), enhanced correlations arise between neutrons and protons (two distinct types of fermions) that occupy orbitals with the same quantum numbers. Such correlations have been predicted to favour an unusual type of nuclear superfluidity, termed isoscalar neutron–proton pairing, in addition to normal isovector pairing. Despite many experimental efforts, these predictions have not been confirmed. Here we report the experimental observation of excited states in the N = Z = 46 nucleus 92Pd. Gamma rays emitted following the 58Ni(36Ar,2n)92Pd fusion–evaporation reaction were identified using a combination of state-of-the-art high-resolution γ-ray, charged-particle and neutron detector systems. Our results reveal evidence for a spin-aligned, isoscalar neutron–proton coupling scheme, different from the previous prediction. We suggest that this coupling scheme replaces normal superfluidity (characterized by seniority coupling) in the ground and low-lying excited states of the heaviest N = Z nuclei. Such strong, isoscalar neutron–proton correlations would have a considerable impact on the nuclear level structure and possibly influence the dynamics of rapid proton capture in stellar nucleosynthesis. ; This work was supported by the Swedish Research Council (contract nos 2007-4067 and 2008-5793), the Göran Gustafsson Foundation, the European Union Sixth Framework Programme 'Integrating Infrastructure Initiative – Transnational Access' (no. 506065; EURONS), the Hungarian Scientific Research Fund, OTKA (contract nos. K72566 and K68801), the UK Science and Technology Facilities Council (STFC), the Polish Ministry of Science and Higher Education (grant no. N N202 073935), the Spanish Ministerio de Ciencia e Innovación (contract no. FPA2007-66069), the Spanish Consolider-Ingenio 2010 Programme CPAN (CSD2007-00042), and Ankara University BIYEP project no. DPT 2005120140. ; Peer reviewed